Changes of nitrogen deposition in China from 1980 to 2018

Wen, Z., Xu, W., Li, Q., Han, M., Tang, A., Zhang, Y., Luo, X., Shen, J., Wang, W., Li, K., +9 more...Pan, Y., Zhang, L., Li, W., Collett, J. L., Zhong, B., Wang, X., Goulding, Keith, Zhang, F. and Liu, X. (2020) Changes of nitrogen deposition in China from 1980 to 2018. Environment International, 144. p. 106022. 10.1016/j.envint.2020.106022
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China has experienced a dramatic change in atmospheric reactive nitrogen (Nr) emissions over the past four decades. However, it remains unclear how nitrogen (N) deposition has responded to increases and/or decreases in Nr emissions. This study quantitatively assesses temporal and spatial variations in measurements of bulk and calculated dry N deposition in China from 1980 to 2018. A long-term database (1980–2018) shows that bulk N deposition peaked in around 2000, and had declined by 45% by 2016–2018. Recent bulk and dry N deposition (based on monitoring from 2011 to 2018) decreased from 2011 to 2018, with current average values of 19.4 ± 0.8 and 20.6 ± 0.4 kg N ha−1 yr−1, respectively. Oxidized N deposition, especially dry deposition, decreased after 2010 due to NOx emission controls. In contrast, reduced N deposition was approximately constant, with reductions in bulk NH4+-N deposition offset by a continuous increase in dry NH3 deposition. Elevated NH3 concentrations were found at nationwide monitoring sites even at urban sites, suggesting a strong influence of both agricultural and non-agricultural sources. Current emission controls are reducing Nr emissions and deposition but further mitigation measures are needed, especially of NH3, built on broader regional emission control strategies.


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